I think you've heard of the cashmere goat farm which is between Castellina and Radda - take a look at their site for info: http://www.chianticashmere.com/en/
As far as places with animals, you want to just visit or stay there? Take a look at Agriturismo Montalbino closer to Monterspertoli, they have a farm with many animals perfect for little kids.
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