Your question makes perfect sense - you want to be somewhere in the middle of these places so that you can move easily between them by train or bus.
Montecatini Terme is a great location, especially if you want to also enjoy the natural springs at the many spas found in the city. But it is a bit further north than Pisa, located along the train line that connects Florence to Lucca. If you wanted to go to Pisa by train, you'd first have to go to Lucca. To go to Siena, on the other hand, you'd have to go to Florence, change trains to Empoli and then change train again to go to Siena.
Therefore, I recommend staying a little further south, closer to the main train line between Florence and Pisa or along the route between Empoli and Siena. It would be good to stay in either Castelfiorentino, Certaldo or even somewhere close to Poggibonsi (not in the town as it has tended to become quite industrial around the edges). The only farmhouse apartment that comes quickly to mind in these towns is Cabbiavoli just outside of Castelfiorentino's city center - check it out to see whether it would meet your needs.






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. Thanks so much in advance 


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